Direct discharge of sewage to natural water through illicitly connected urban stormwater systems: An overlooked source of dissolved organic matter

Ruihua Zhang, Rong Xiao, Feifei Wang, Wenhai Chu*, Jinglong Hu, Yu Zhang, Wei Jin, Jan Peter van der Hoek, Zuxin Xu

*Corresponding author for this work

Research output: Contribution to journalArticleScientificpeer-review

13 Downloads (Pure)

Abstract

The illicit connection of sewage pipes to stormwater pipes commonly occurs in urban stormwater systems. This brings problems that sewage might be directly discharges into natural water and even drinking water sources without treatment, posing risks to ecological safety. Sewage contains various unknown dissolved organic matter (DOM), which could react with disinfectants and lead to the formation of carcinogenic disinfection byproducts (DBPs). Thus, understanding the impacts of illicit connections on downstream water quality is of significance. This study firstly investigated the characteristics of DOM using fluorescence spectroscopy and the formation of DBPs after chlorination in an urban stormwater drainage system in the case of illicit connections. The results found that the concentrations of dissolved organic carbon and dissolved organic nitrogen ranged from 2.6 to 14.9 mg/L and from 1.8 to 12.6 mg/L, respectively, with the highest levels occurring at the illicit connection points. Concerning DBP precursors, pipe illicit connections introduced considerable precursors of highly toxic haloacetaldehydes and haloacetonitriles into the stormwater pipes. Furthermore, illicit connections introduced more contents of tyrosine-like and tryptophan-like aromatic proteins, which may be related to foods, nutrients, personal care products, etc. in the untreated sewage. This indicated that the urban stormwater drainage system was a significant input source of DOM and DBP precursors to natural water. The results of this study are of great significance for protecting the security of water sources and promoting the sustainability of urban water environment.
Original languageEnglish
Article number164248
Number of pages10
JournalScience of the Total Environment
Volume890
DOIs
Publication statusPublished - 2023

Bibliographical note

Green Open Access added to TU Delft Institutional Repository ‘You share, we take care!’ – Taverne project https://www.openaccess.nl/en/you-share-we-take-care
Otherwise as indicated in the copyright section: the publisher is the copyright holder of this work and the author uses the Dutch legislation to make this work public.

Keywords

  • Disinfection byproducts
  • Dissolved organic matter
  • Illicit connection
  • Precursors
  • Urban stormwater system

Fingerprint

Dive into the research topics of 'Direct discharge of sewage to natural water through illicitly connected urban stormwater systems: An overlooked source of dissolved organic matter'. Together they form a unique fingerprint.

Cite this