TY - JOUR
T1 - Effective Approaches of Improving the Performance of Chalcogenide Solid Electrolytes for All-Solid-State Sodium-Ion Batteries
AU - Dai, Hanqing
AU - Xu, Wenqian
AU - Hu, Zhe
AU - Chen, Yuanyuan
AU - Wei, Xian
AU - Yang, Bobo
AU - Chen, Zhihao
AU - Gu, Jing
AU - Yang, Dan
AU - Xie, Fengxian
AU - Zhang, Wanlu
AU - Guo, Ruiqian
AU - Zhang, Guoqi
AU - Wei, Wei
PY - 2020
Y1 - 2020
N2 - All-solid-state sodium-ion batteries (SIBs) possess the advantages of rich resources, low price, and high security, which are one of the best alternatives for large-scale energy storage systems in the future. Also, the chalcogenide solid electrolytes (CSEs) of SIBs have the characteristics of excellent room-temperature ionic conductivity (10−3-10−2 S cm−1), low activation energy (<0.6 eV), easy cold-pressing consolidation, etc. Hence, CSEs have become a very active area of all-solid-state SIB research in recent years. In this review, the modification methods and implementation technologies of CSEs are summarized, and the structure and electrochemical performance of the CSEs are discussed. Furthermore, the auxiliary function of first-principle calculations for modification is introduced. Ultimately, we describe the challenges regarding CSEs and propose some strategic suggestions.
AB - All-solid-state sodium-ion batteries (SIBs) possess the advantages of rich resources, low price, and high security, which are one of the best alternatives for large-scale energy storage systems in the future. Also, the chalcogenide solid electrolytes (CSEs) of SIBs have the characteristics of excellent room-temperature ionic conductivity (10−3-10−2 S cm−1), low activation energy (<0.6 eV), easy cold-pressing consolidation, etc. Hence, CSEs have become a very active area of all-solid-state SIB research in recent years. In this review, the modification methods and implementation technologies of CSEs are summarized, and the structure and electrochemical performance of the CSEs are discussed. Furthermore, the auxiliary function of first-principle calculations for modification is introduced. Ultimately, we describe the challenges regarding CSEs and propose some strategic suggestions.
KW - chalcogenide solid electrolytes
KW - electrochemical performance
KW - first-principle calculations
KW - modification methods
KW - sodium-ion batter
UR - http://www.scopus.com/inward/record.url?scp=85087148240&partnerID=8YFLogxK
U2 - 10.3389/fenrg.2020.00097
DO - 10.3389/fenrg.2020.00097
M3 - Review article
AN - SCOPUS:85087148240
SN - 2296-598X
VL - 8
SP - 1
EP - 7
JO - Frontiers in Energy Research
JF - Frontiers in Energy Research
M1 - 97
ER -