Efficient Aerobic Oxidation of trans-2-Hexen-1-ol using the Aryl Alcohol Oxidase from Pleurotus eryngii

T. P. de Almeida; M. M.C.H. van Schie; A. Ma; F. Tieves; S. H.H. Younes; E. Fernández-Fueyo; I. W.C.E. Arends; A. Riul; F. Hollmann

doi:10.1002/adsc.201801312

Efficient Aerobic Oxidation of trans-2-Hexen-1-ol using the Aryl Alcohol Oxidase from Pleurotus eryngii

T. P. de Almeida, M. M.C.H. van Schie, A. Ma, F. Tieves, S. H.H. Younes, E. Fernández-Fueyo, I. W.C.E. Arends, A. Riul, F. Hollmann^*

^*Corresponding author for this work

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Abstract

The selective oxidation of trans-2-hexen-1-ol to the corresponding aldehyde using a recombinant aryl alcohol oxidase from Pleurotus eryngii (PeAAOx) is reported. Especially using the two liquid phase system to overcome solubility and product inhibition issues enabled to achieve more than 2.200.000 catalytic turnovers for the production enzyme as well as molar product concentrations, pointing towards an economic feasible reaction.

Original language	English
Pages (from-to)	2668-2672
Number of pages	5
Journal	Advanced Synthesis and Catalysis
Volume	361
Issue number	11
DOIs	https://doi.org/10.1002/adsc.201801312
Publication status	Published - 2019

Keywords

biocatalysis
oxidase
oxidation reactions
two liquid phase system

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title = "Efficient Aerobic Oxidation of trans-2-Hexen-1-ol using the Aryl Alcohol Oxidase from Pleurotus eryngii",

abstract = "The selective oxidation of trans-2-hexen-1-ol to the corresponding aldehyde using a recombinant aryl alcohol oxidase from Pleurotus eryngii (PeAAOx) is reported. Especially using the two liquid phase system to overcome solubility and product inhibition issues enabled to achieve more than 2.200.000 catalytic turnovers for the production enzyme as well as molar product concentrations, pointing towards an economic feasible reaction.",

keywords = "biocatalysis, oxidase, oxidation reactions, two liquid phase system",

author = "{de Almeida}, {T. P.} and {van Schie}, {M. M.C.H.} and A. Ma and F. Tieves and Younes, {S. H.H.} and E. Fern{\'a}ndez-Fueyo and Arends, {I. W.C.E.} and A. Riul and F. Hollmann",

year = "2019",

doi = "10.1002/adsc.201801312",

language = "English",

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journal = "Advanced Synthesis and Catalysis",

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T1 - Efficient Aerobic Oxidation of trans-2-Hexen-1-ol using the Aryl Alcohol Oxidase from Pleurotus eryngii

AU - de Almeida, T. P.

AU - van Schie, M. M.C.H.

AU - Ma, A.

AU - Tieves, F.

AU - Younes, S. H.H.

AU - Fernández-Fueyo, E.

AU - Arends, I. W.C.E.

AU - Riul, A.

AU - Hollmann, F.

PY - 2019

Y1 - 2019

N2 - The selective oxidation of trans-2-hexen-1-ol to the corresponding aldehyde using a recombinant aryl alcohol oxidase from Pleurotus eryngii (PeAAOx) is reported. Especially using the two liquid phase system to overcome solubility and product inhibition issues enabled to achieve more than 2.200.000 catalytic turnovers for the production enzyme as well as molar product concentrations, pointing towards an economic feasible reaction.

AB - The selective oxidation of trans-2-hexen-1-ol to the corresponding aldehyde using a recombinant aryl alcohol oxidase from Pleurotus eryngii (PeAAOx) is reported. Especially using the two liquid phase system to overcome solubility and product inhibition issues enabled to achieve more than 2.200.000 catalytic turnovers for the production enzyme as well as molar product concentrations, pointing towards an economic feasible reaction.

KW - biocatalysis

KW - oxidase

KW - oxidation reactions

KW - two liquid phase system

UR - http://www.scopus.com/inward/record.url?scp=85061275748&partnerID=8YFLogxK

U2 - 10.1002/adsc.201801312

DO - 10.1002/adsc.201801312

M3 - Article

AN - SCOPUS:85061275748

SN - 1615-4150

VL - 361

SP - 2668

EP - 2672

JO - Advanced Synthesis and Catalysis

JF - Advanced Synthesis and Catalysis

IS - 11

ER -

Efficient Aerobic Oxidation of trans-2-Hexen-1-ol using the Aryl Alcohol Oxidase from Pleurotus eryngii

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Keywords

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