TY - JOUR
T1 - Competing soft phonon modes at the charge-density-wave transitions in DyT e3
AU - Maschek, M.
AU - Zocco, D. A.
AU - Rosenkranz, S.
AU - Heid, R.
AU - Said, Ayman. H.
AU - Alatas, A.
AU - Walmsley, P.
AU - Fisher, I. R.
AU - Weber, F.
PY - 2018
Y1 - 2018
N2 - The family of rare-earth (R) tritellurides RTe3 features charge-density-wave (CDW) order related to strongly momentum-dependent electron-phonon coupling. Similar to other CDW compounds, superconductivity is observed when the CDW order is suppressed via hydrostatic pressure [J. J. Hamlin, Phys. Rev. Lett. 102, 177002 (2009)10.1103/PhysRevLett.102.177002]. What sets the heavier members of the RTe3 series apart is the observation of a second CDW transition at lower temperatures having an in-plane ordering wave vector qCDW,2 [100] of almost the same magnitude but orthogonal to the ordering wave vector qCDW,1 [001] observed at higher temperatures [N. Ru, Phys. Rev. B 77, 035114 (2008)10.1103/PhysRevB.77.035114]. Here, we report an inelastic x-ray scattering investigation of the lattice dynamics of DyTe3 In particular, we show that there are several phonon modes along both in-plane directions, which respond to the onset of the CDW transition at TCDW,1=308K. Surprisingly, these soft modes close to qCDW,2=(0.68,0,0) show strong softening near TCDW,1 but do not exhibit any response to the lower-temperature transition at TCDW,2=68K. Our results indicate that the low-temperature CDW order is not just the 90° rotated analogue of the one appearing at high temperatures.
AB - The family of rare-earth (R) tritellurides RTe3 features charge-density-wave (CDW) order related to strongly momentum-dependent electron-phonon coupling. Similar to other CDW compounds, superconductivity is observed when the CDW order is suppressed via hydrostatic pressure [J. J. Hamlin, Phys. Rev. Lett. 102, 177002 (2009)10.1103/PhysRevLett.102.177002]. What sets the heavier members of the RTe3 series apart is the observation of a second CDW transition at lower temperatures having an in-plane ordering wave vector qCDW,2 [100] of almost the same magnitude but orthogonal to the ordering wave vector qCDW,1 [001] observed at higher temperatures [N. Ru, Phys. Rev. B 77, 035114 (2008)10.1103/PhysRevB.77.035114]. Here, we report an inelastic x-ray scattering investigation of the lattice dynamics of DyTe3 In particular, we show that there are several phonon modes along both in-plane directions, which respond to the onset of the CDW transition at TCDW,1=308K. Surprisingly, these soft modes close to qCDW,2=(0.68,0,0) show strong softening near TCDW,1 but do not exhibit any response to the lower-temperature transition at TCDW,2=68K. Our results indicate that the low-temperature CDW order is not just the 90° rotated analogue of the one appearing at high temperatures.
UR - http://www.scopus.com/inward/record.url?scp=85053406928&partnerID=8YFLogxK
U2 - 10.1103/PhysRevB.98.094304
DO - 10.1103/PhysRevB.98.094304
M3 - Article
AN - SCOPUS:85053406928
SN - 2469-9950
VL - 98
JO - Physical Review B
JF - Physical Review B
IS - 9
M1 - 094304
ER -