Performance improvement by alumina coatings on Y3Al5O12: Ce3+ phosphor powder deposited using atomic layer deposition in a fluidized bed reactor

Zhi Zhou, Nan Zhou, Xiangyang Lu, Melvin Ten Kate, D. Valdesueiro Gonzalez, J.R. van Ommen, H. T. Hintzen

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To improve the thermal stability, Al2O3 has been successfully coated on a Y3Al5O12:Ce3+ (YAG:Ce) phosphor powder host by using the Atomic Layer Deposition (ALD) approach in a fluidized bed reactor. Transmission Electron Microscopy (TEM) and Energy Dispersive X-ray spectroscopy (EDX) analysis indicate that coating an Al2O3 thin layer by ALD is highly feasible. The luminescence properties (such as excitation and emission as well as quantum efficiency and UV-absorption of the coated YAG:Ce phosphor) were systematically analysed, with the further examination of the thermal resistance characteristics. The Al2O3 thin layer coating with precisely controlled thickness by ALD can obviously improve the luminescence intensity and greatly enhances the thermal stability of the YAG:Ce phosphor. It is suggested that the alumina coating with tailoring thickness seems not only to act like a barrier to decrease the thermal quenching, but also as a great help to promote the light absorption and transfer.

Original languageEnglish
Pages (from-to)76454-76462
Number of pages9
JournalRSC Advances
Issue number80
Publication statusPublished - 2016

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