Synthesis of hierarchical zeolites using an inexpensive mono-quaternary ammonium surfactant as mesoporogen

Xiaochun Zhu; Roderigh Rohling; Georgy Filonenko; Brahim Mezari; Jan P. Hofmann; Shunsuke Asahina; Emiel J.M. Hensen

doi:10.1039/c4cc06267a

Synthesis of hierarchical zeolites using an inexpensive mono-quaternary ammonium surfactant as mesoporogen

Xiaochun Zhu, Roderigh Rohling, Georgy Filonenko, Brahim Mezari, Jan P. Hofmann, Shunsuke Asahina, Emiel J.M. Hensen^*

^*Corresponding author for this work

Research output: Contribution to journal › Article › Scientific › peer-review

50 Citations (Scopus)

Abstract

A simple amphiphilic surfactant containing a mono-quaternary ammonium head group (N -methylpiperidine) is effective in imparting substantial mesoporosity during synthesis of SSZ-13 and ZSM-5 zeolites. Highly mesoporous SSZ-13 prepared in this manner shows greatly improved catalytic performance in the methanol-to-olefins reaction compared to bulk SSZ-13.

Original language	English
Pages (from-to)	14658-14661
Journal	Chemical Communications
Volume	50
Issue number	93
DOIs	https://doi.org/10.1039/c4cc06267a
Publication status	Published - 2014
Externally published	Yes

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abstract = "A simple amphiphilic surfactant containing a mono-quaternary ammonium head group (N -methylpiperidine) is effective in imparting substantial mesoporosity during synthesis of SSZ-13 and ZSM-5 zeolites. Highly mesoporous SSZ-13 prepared in this manner shows greatly improved catalytic performance in the methanol-to-olefins reaction compared to bulk SSZ-13.",

author = "Xiaochun Zhu and Roderigh Rohling and Georgy Filonenko and Brahim Mezari and Hofmann, {Jan P.} and Shunsuke Asahina and Hensen, {Emiel J.M.}",

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T1 - Synthesis of hierarchical zeolites using an inexpensive mono-quaternary ammonium surfactant as mesoporogen

AU - Zhu, Xiaochun

AU - Rohling, Roderigh

AU - Filonenko, Georgy

AU - Mezari, Brahim

AU - Hofmann, Jan P.

AU - Asahina, Shunsuke

AU - Hensen, Emiel J.M.

PY - 2014

Y1 - 2014

N2 - A simple amphiphilic surfactant containing a mono-quaternary ammonium head group (N -methylpiperidine) is effective in imparting substantial mesoporosity during synthesis of SSZ-13 and ZSM-5 zeolites. Highly mesoporous SSZ-13 prepared in this manner shows greatly improved catalytic performance in the methanol-to-olefins reaction compared to bulk SSZ-13.

AB - A simple amphiphilic surfactant containing a mono-quaternary ammonium head group (N -methylpiperidine) is effective in imparting substantial mesoporosity during synthesis of SSZ-13 and ZSM-5 zeolites. Highly mesoporous SSZ-13 prepared in this manner shows greatly improved catalytic performance in the methanol-to-olefins reaction compared to bulk SSZ-13.

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U2 - 10.1039/c4cc06267a

DO - 10.1039/c4cc06267a

M3 - Article

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VL - 50

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JO - Chemical Communications

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ER -

Synthesis of hierarchical zeolites using an inexpensive mono-quaternary ammonium surfactant as mesoporogen

Abstract

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